canon is right, it's Doolittle. I don't think Surfer Rosa comes close. guitars are too quiet. too much relative filler. best drum sound though, fair enough.
the other two aren't as good on the whole, but have the best songs among their ranks ('Velouria', 'Dig For Fire', 'Alec Eiffel', 'Motorway to Roswell').
can't believe I'm starting a Pixies topic. oh well, have at it.