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...is the most accessible of their really good albums.
The 40 licks best of is a must buy too. (As long as you skip the tracks recorded in the last 20 years.)
exile on main st
let it bleed
would be that album
40 Licks has some more recent and rubbish stuff, 80's Stones etc...Hot Rocks has all the essential tracks.
All the other aforementioned albums are ace...
3cd collection "The London Years".
It covers all the stuff from the start right up to about 1971. Then investigate the individual albums Beggars Banquet, Let It Bleed, Sticky Fingers and Exile on Main Street.